Advances in Chemical Physics, Volume 158: Physical Chemistry by Mitsuru Nagasawa

By Mitsuru Nagasawa

The Advances in Chemical Physics sequence offers the chemical physics box with a discussion board for serious, authoritative reviews of advances in each zone of the self-discipline. This quantity explores issues from Thermodynamic houses of Polyelectrolyte options to ion-binding of polyelectrolytes. The booklet features:

  • The basically sequence of volumes to be had that offers the leading edge of analysis in chemical physics
  • Contributions from specialists during this box of research
  • Representative cross-section of study that questions proven considering on chemical solutions
  • An editorial framework that makes the booklet an exceptional complement to a sophisticated graduate classification in actual chemistry or chemical physics

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MITSURU NAGASAWA 32 107 106 M S 105 C D 104 10–2 10–1 1 3 C (g/cm ) Figure 6. Molecular weight–concentration diagram for three regions. D, S, and C denote dilute, semidilute, and concentrated solution regions, respectively. Sample; poly(styrene) with NMWD. Solvent, toluene or benzene. (Reproduced with permission from Ref. [23]. ) II. ELECTROSTATIC FREE ENERGY OF POLYELECTROLYTE SOLUTIONS In aqueous solutions of a strong electrolyte of uni–univalent type K + A− , the Gibbs free energy G of the solution at constant pressure and temperature may be expressed by dGT,P = ????+ dn+ + ????− dn− + ????o dno (19) where ????i and ni denote the chemical potential and the concentration (mol/l) of species i, respectively.

15, 1129 (1977). 32. J. G. Kirkwood and R. J. Goldberg, J. Chem. , 18, 54 (1950). INTRODUCTORY REMARKS 33. 34. 35. 36. 37. 38. 39. 40. 41. 42. 43. 44. 45. 19 W. H. Stockmayer, J. Chem. , 18, 58 (1950). E. F. Casassa and H. Eisenberg, J. Phys. , 64, 753 (1960); 65, 427 (1961). H. Eisenberg and E. F. Casassa, J. Polym. , 47, 29 (1960). H. Eisenberg, J. Chem. , 36, 1837 (1962). A. Vrij and J. Th. G. Overbeek, J. , 17, 944 (1962). A. Takahashi, T. Kato and M. Nagasawa, J. Phys. , 71, 2001 (1967).

Reproduced with permission from Ref. [47]. ) Section “Polymer√ Science”). The values obtained are plotted against (A) 1∕Cs and (B) 1∕ Cs in Figure 12. The values of A2,OS are indicated by cross, while A2,LS values indicated by circles. Both A2,OS and A2,LS are found to be almost identical, despite that the NaPSS samples were prepared by fractionation, so having broad molecular weight distributions. The identity of A2,OS and A2,LS may arise from the fact that the second virial coefficient of NaPSS does not depend on molecular weight in this range of added-salt concentration, as is observed in Figure 13.

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